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She makes the move after filming of Brad Pitt's movie runs over its schedule.
Brad and his brood are in the UK whilst he films his latest movie World War Z and due to it being behind schedule the pair have enrolled their children at a Primary school in Richmond, West London.
A source told The Sun: "The children are home tutored in the United States. But wherever possible Brad and Angelina like to have them attend local schools to introduce them to the culture of each country."
Brad's latest flick is an apocalyptic zombie horror and you can see some behind-the-scenes shots on-set below...